You should have really asked "What actor would be the best at scaring the pants off of you" because certain actors just ooze evil, Jack Nicholson for example is just as scary in The Shining as he is in Batman, and even more sinister in The Departed because he's supposed to be sane.
Can't think of many other actors that have got that "Look at me, I'm cool AND evil and you so want to be me" act down to a T, although Michael Keaton did sort of give me the willies in Pacific Heights because, again, he plays that sort of deranged but perfectly sane character with such ease.
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